Chichibabin reaction

Chichibabin reaction
Named after Aleksei Chichibabin
Reaction type Substitution reaction
Identifiers
RSC ontology ID RXNO:0000527

The Chichibabin reaction (pronounced ' (chē')-chē-bā-bēn) is a method for producing 2-aminopyridine derivatives by the reaction of pyridine with sodium amide. It was reported by Aleksei Chichibabin in 1914. The following is the overall form of the general reaction:

The direct amination of pyridine with sodium amide can take place in liquid ammonia or an aprotic solvent such as xylene is commonly used. Following the addition elimination mechanism first a nucleophilic NH2 is added while a hydride (H) is leaving. The reaction formally is a nucleophilic substitution of hydrogen SNH.

Ciganek describes an example of an intramolecular Chichibabin reaction in which a nitrile group on a fused ring is the source of nitrogen in amination.